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Lösungsmittel-, Viskositäts-, Säure- und Substituenteneinflüsse auf die Photoisomerisierung und Relaxation symmetrischer Triazacarbocyanine bei 283 bis 323 K

✍ Scribed by Heinz Balli; Bruno Hellrung


Publisher
John Wiley and Sons
Year
1985
Tongue
German
Weight
259 KB
Volume
68
Category
Article
ISSN
0018-019X

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✦ Synopsis


Influence of Solvents, Viscosity, Acid, and Substituents on the Photoisomerization and the Relaxation of Symmetrical Triazacarbocyanine Dyes at 283 to 323 K

Photobleaching and the reverse dark reaction of seven symmetrical triazacarbocyanine dyes with different heterocycles were studied dependent on solvent effects (protic and aprotic solvents), on effects of viscosity (glycerol/EtOH mixtures), and on effects of added acid. No effects of dissolved O~2~ or added I~2~ has been observed. Kinetic data (Δ__H__^≠^, Δ__S__^≠^, and Δ__G__) of the reverse reaction are given. The effect of the substituents has been studied on two series of substituted triazacarbocyanine dyes. The mechanism of the reverse reaction is discussed.