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Luminescence Stimulated by Electron Transfer: Fluorescent Donor/Acceptor-Substituted Stilbenes Containing Pyrenoid and Heteroaromatic Subunits

✍ Scribed by Dr. Andreas Knorr; Prof. Dr. Jörg Daub


Publisher
John Wiley and Sons
Year
1996
Tongue
English
Weight
327 KB
Volume
34
Category
Article
ISSN
0044-8249

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✦ Synopsis


a = 88.89(3), fi = 89.14(2), y = 61.85(2)", V = 8070(5) A', Z = 2, p,,,, =1.353 M ~I I -~, E. = 0.71073 A, T=153 K, p(Mo,,) = 0.679 mm-'. Data was collected on a Siemens-Stoe AED diffractometer using an oil-coated, rapidly cooled crystal of dimensions 0.4 x 0.3 x 0.3 mm mounted directly from solution 1131; S/w method (5" 5 20 5 45"). The data were corrected for absorption by a semiempirical method based upon P-scan data with maximum and minimum transmission of 0.908 and 0.775, respectively. Of 21 897 reflections collected, 21 131 were independent. The structure was solved by direct methods (SHELXTL PLUS) and refined by full matrix least squares on F 2 ; R1 [F > 4a(F)] and wR2 (all data) to 0.0729 and 0.1656, respectively (SHELXL-93, Gottingen, 1993). All the non-hydrogen atoms in the anion of 1 were refined with anisotropic displacement parameters. One of the [Li(thf),]+ cations and 3.5 of the 5.5 independent noncoordinated T H F molecules are disordered on two positions, halfof them on the inversion center. All five non-hydrogen atoms ofeach T H F molecule in the unit cell were refined with the same isotropic parameters and distance restraints. Hydrogen atoms were set geometrically. Maximum and minimum residual electron density in the final difference map. 2.018 and -1.103 e k 3 . respectively. Further details of the crystal structure investigation may he obtained from the