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Low frequency elastic modulus measurements on segmented ester polyurethanes

✍ Scribed by A.R. Eastwood; R.A. Pethrick


Publisher
Elsevier Science
Year
1983
Tongue
English
Weight
406 KB
Volume
19
Category
Article
ISSN
0014-3057

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✦ Synopsis


Low frequency extentional modulus measurements are reported as a function of temperature on a series of low isocyanate containing segmented ethyleneadipate diphenyldiisocyanate elastomers. The effects of variation of isocyanate content, molecular weight of the ester block and the ratio of 1, 3 to 1, 4 butanediol chain extender on thc glass transition temperatures of the ester phase are explored. The mobility of ~he ester phase appears to reflect the degree of perfection of the organisation of the urethane phase. The plateau modulus similarly exhibits a correlation with the perfection of the hard phase packing and this is also reflected in the variation of the effective crosslink density obtained from swell measurements. The detailed organisation appears from this study to influence the degree of mobility of the ester phase.