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Low-Coordinate Arsenic Chemistry: Studies of Amino(iminoarsanes) Using UV Photoelectron Spectroscopy and Density Functional Theory

✍ Scribed by Karinne Miqueu; J.-M. Sotiropoulos; G. Pfister-Guillouzo; V. Romanenko

Publisher: John Wiley and Sons
Year: 2000
Tongue: English
Weight: 370 KB
Volume: 2000
Category: Article
ISSN: 1434-1948
DOI: 10.1002/(sici)1099-0682(200003)2000:3<477::aid-ejic477>3.0.co;2-n

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✦ Synopsis

In this paper, we report the gas-phase characterization of two differently substituted amino(iminoarsanes), TmpAs= NSiMe 3 and (SiMe 2 tBu) 2 NAs=N(SiMe 2 tBu), by coupling flash vacuum thermolysis (FVT) with UV photoelectron spectroscopy (PES). Quantum chemical calculations, using the DFT method (B3LYP) with the basis set 6-311G(d,p), have

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