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Long-range 1H coupling interactions: Identification of different pathways by 2D NMR δ—δ correlated spectroscopy. Applications in structural analysis

✍ Scribed by N. Platzer; N. Goasdoue; D. Davoust


Publisher
John Wiley and Sons
Year
1987
Tongue
English
Weight
740 KB
Volume
25
Category
Article
ISSN
0749-1581

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✦ Synopsis


The simplest methods of 2D 6-6 correlated spectroscopy (COSY and COSY LR) allow the easy observation of long-range coupling interactions. It is shown how these methods can lead to the discrimination between different pathways across single bonds: 4J through coplanar or gauche arrangement of the bonds and ' J through a zig-zag pathway or bond proximity. Applications to configurational and conformational analysis of polycyclic compounds, a trimer of isophorone, two natural terpenoids (carotol and daucol) and four steroids, are presented.