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Local Viscosity in the Vicinity of a Wall Coated by Polymer Brush from Green–Kubo Relations

✍ Scribed by Dimitar I. Dimitrov; Andrey Milchev; Kurt Binder


Publisher
John Wiley and Sons
Year
2008
Tongue
English
Weight
372 KB
Volume
17
Category
Article
ISSN
1022-1344

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✦ Synopsis


Abstract

When fluids are confined in slit pores between parallel walls, their static structures and their dynamical properties exhibit inhomogeneity in the z‐direction perpendicular to the wall. Of particular interest are local bulk viscosity η~b~(z) and shear viscosity η~s~(z). Here, we discuss an algorithm to estimate these quantities from Green–Kubo relations using equilibrium molecular dynamics. As an application example, a polymer brush (macromolecules end‐grafted to a substrate at z = 0) interacting with a solvent formed from point‐like particles is given.

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