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Liquid crystal control. A remarkable enhancement of both efficiency and diastereoselectivity of intramolecular thermal cycloadditions in smectic solvents

✍ Scribed by Kenji Fukunaga; Takehisa Kunieda


Book ID
104261983
Publisher
Elsevier Science
Year
1999
Tongue
French
Weight
243 KB
Volume
40
Category
Article
ISSN
0040-4039

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✦ Synopsis


The uncatalyzcd intramolecular [4+2]cycloaddition of 2E,TE,9(E)-decatrienoates, conducted at 140 oC in a medium of smectic liquid cryctals proceeds with a remarkably high level of chendcai efficiency and diastereselectivity, in contrast to the isotropic phase reactions which result in much lower yield and selectivity.