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Linewidth dependence of quasi-stationary states in large molecules

✍ Scribed by C. Tric

Publisher
Elsevier Science
Year
1973
Tongue
English
Weight
506 KB
Volume
21
Category
Article
ISSN
0009-2614

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✦ Synopsis

Recerved 2 Apr11 1973

We study the quaskstatlonary state?, or elgenstates, of the decay matrlv for a system described by one su-igle VIbromc state 1s) coupled to a marufold (I), both Is) and (I} levels bemg coupled to separate contmua whrch endow them with fuute lmeuldths rs, r[ When all the zero-order states have the same 1JneWJdth (not necessartiy zero) the quasi-stationary states are ldentlcai to the molecular eIgenstatcs, when the difference between the lmewldths 7x_ 71 IS large enough, the zero-order sctp (s, {I}) are comp!etely decoupled, a result which has been establrsbed for the twolevel system We mdlcote some consequences of colhslonal broadenmg mvolvmg pressure effects m the gas phase

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