Linear and Nonlinear Optical Spectroscopy and Microscopy (Progress in Optical Science and Photonics, 29)

✍ Scribed by Mengtao Sun, Xijiao Mu, Rui Li

• Publisher: Springer
• Year: 2024
• Tongue: English
• Leaves: 125
• Category: Library

✦ Synopsis

The nonlinear optical spectrum signal technology is a new type of optical characterization technology owing to its non-invasiveness and good biocompatibility. This book highlights a comprehensive introduction to the Stimulated Raman scattering (SRS), Anti-Stokes Raman Spectroscopy (CARS), Two-photon Excited Fluorescence (TPEF) and Second Harmonic Generation signals (SHG) technologies. The four types of nonlinear optical signals technologies, especially two-dimensional and three-dimensional imaging, have great application potential in physics, materials science, chemistry and biomedicine. The book covers principles, theoretical calculation methods, signal measurement methods and imaging specific methods. The theoretical part starts from the basics of nonlinear optics and the relationship with strong light, and gradually transitions to theoretical calculation methods for specific optical signals. it combines the classical theory and the quantum theory to help readers develop a thorough understanding of the technologies. The book is a good reference for graduate students majored in physics and chemistry and for researchers working on optics, photonics and materials science.

✦ Table of Contents

Contents
1 Introduction
2 Basic Theory of Nonlinear Optics
2.1 Classical Electromagnetic Theory of Nonlinear Optics
2.1.1 Measurement of Nonlinear Optical Processes
2.1.2 Nonlinear Induced Polarization Effect of Optical Media
2.1.3 Tensor Representation of Nonlinear Polarization
2.1.4 Rotational Symmetry of Nonlinear Polarizability Tensor Elements
2.1.5 Time Reversal Symmetry of Polarization Rate
2.2 Quantum Theory and Method of Nonlinear Optics
2.2.1 Density Matrix
2.2.2 Time-Dependent Density Matrix
2.2.3 The Tensor and Properties of the Polarizability of the Independent Molecular System
2.2.4 The Tensor and Properties of the Polarizability of the Molecular System with Inter-molecular Interaction
2.2.5 Resonance Enhanced Polarizability
2.2.6 Calculation Method of Nonlinear Polarizability by Higher-Order Derivative
2.2.7 Nonlinear Polarizability by Sum-Over-States (SOS) Method
2.3 Common Nonlinear Optical Processes
2.3.1 Second-Harmonic Generation (SHG)
2.3.2 Sum-Frequency Generation (SFG)
2.3.3 Raman Amplification
2.3.4 Four-Wave Mixing
3 The Principle, Application and Imaging of CARS
3.1 Principles of CARS
3.1.1 Mechanism of CARS Signal Generation
3.1.2 CARS Optical Configuration
3.2 Biomedical Imaging of CARS
3.2.1 Lipid
3.3 Materials Imaging of CARS
3.3.1 CARS Image for Porous Carbon
3.3.2 CARS Image for Graphene
4 The Principle, Application and Imaging of SRS
4.1 Principles of SRS
4.1.1 Quantum Theory of SRS
4.1.2 Instrumentation of SRS
4.2 Biomedical Imaging
4.2.1 SRS Imaging of Hela Cells
4.2.2 SRS Detection and Diagnosis of the Boundary of Glioma
4.2.3 SRS Imaging of Laryngeal Cancer
4.3 Material Composition Analysis
5 The Principle, Application and Imaging of SHG
5.1 Principles of SHG
5.1.1 SHG Optical Configuration
5.2 Biomedical Imaging of SHG
5.2.1 Collagen
5.2.2 SHG Imaging for Elastic Arteries
5.2.3 SHG Imaging for Snail
6 The Principle, Application and Imaging of TPEF
6.1 Principles of TPEF
6.1.1 Two-Photon Absorption
6.1.2 Design of Strong Two-Photon Absorption Cross Section
6.1.3 Two-Photon Excited/Emitted Fluoresence
6.1.4 TPEF Optical Configuration
6.2 Biomedical Imaging of TPEF
6.2.1 TPEF and Lifetime Imaging for Glioma
6.2.2 TPEF and Lifetime Imaging for Gastrointestinal Cancer
7 The Principle, Application and Imaging of STED
7.1 Principles of STED
7.1.1 Selection of Excitation and Loss Laser Types
7.1.2 Selection of Excitation and Loss Wavelengths
7.2 Biomedical Imaging of STED
7.2.1 Nervous Structure Imaging
7.2.2 3D STED Imaging
8 Plasmon Enhanced Nonlinear Spectroscopy and Imaging
8.1 Principles
8.1.1 Plasmon
8.1.2 Enhancement Mechanism
8.2 Application of Surface Plasmon Enhanced Nonlinear Optical Signals
8.2.1 Surface Plasmon Enhanced CARS
8.2.2 Surface Plasmon Enhanced TPEF
8.2.3 Surface Plasmon Enhanced High-Order Harmonic Wave Generate
Appendix References