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Kinetics of reactions of Schiff base complexes of iron(II). V. Reactions of the complex of the hexadentate ligand NN‴-bis-[α-(2-pyridyl)benzylidene]triethylenetetramine in acid solution and with hydroxide, cyanide, and peroxodisulphate

✍ Scribed by E. R. Gardner; F. M. Mekhail; J. Burgess


Publisher
John Wiley and Sons
Year
1974
Tongue
English
Weight
498 KB
Volume
6
Category
Article
ISSN
0538-8066

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✦ Synopsis


Abstract

The preparation and characterization of the iron(II) complex of the hexadentate Schiff base ligand NN‴‐bis‐[α‐(2‐pyridyl)benzylidene]triethylenetetramine are reported. Kinetic patterns and rate constants for aquation of this complex, and for its reactions with hydroxide, cyanide, and peroxodisulphate have been determined. Activation parameters for the reaction with cyanide, in aqueous solution, are Δ__H__‡ = 24.3 kcal/mole and Δ__S__‡ = +1 cal/deg‐mole.