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Investigation of the hydrogen mobility in a mixed perovskite: Ba[Ca(1+x)/3Nb(2−x)/3]O3−x/2 by quasielastic neutron scattering

✍ Scribed by M. Pionke; T. Mono; W. Schweika; T. Springer; H. Schober

Publisher
Elsevier Science
Year
1997
Tongue
English
Weight
578 KB
Volume
97
Category
Article
ISSN
0167-2738

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✦ Synopsis

Quasielastic neutron scattering was applied to investigate the protonic motion in water-doped Ba[Ca Nb ]O 0.39 0.61 2.91 between 5 and 700 K. The backscattering spectra in the meV-region for small scattering vectors Q lead to the protonic self-diffusion constant. The results were compared with measurements of the electrical conductivity. At larger Q, the spectra reveal two superimposed quasielastic components probably related to two groups of jump rates. Low resolution measurements indicate a rapid rotation of the hydroxyl groups.

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