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Intramolecular reactions of acyclic n-acyliminium ions III silicon assisted cyclocondensation of glyoxylic esters to proline and pipecolic acid derivatives

✍ Scribed by Hendrik H Mooiweer; Henk Hiemstra; Hendrikus P Fortgens; W.Nico Speckamp


Book ID
104227227
Publisher
Elsevier Science
Year
1987
Tongue
French
Weight
267 KB
Volume
28
Category
Article
ISSN
0040-4039

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✦ Synopsis


Cyclizations of acyclic N-acyliminium ions, generated from the adducts of formaldehyde, n-butyl glyoxylate or methyl glyoxylate with amines containing an ally1 or propargyl silane as terminator, lead to 3-ethenyl and 3-ethenylidene substituted pyrrolidines and piperidines, some of which are structurally related to proline and pipecolic acid.