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Intramolecular Hydroaminations Mediated by Reductive Mercuration or n-Butyllithium To Afford 3-Methyl- and 3,4-Dimethyl-1,2,3,4-tetrahydroisoquinolines

✍ Scribed by Rakhi Pathak; Prevashni Naicker; Warren A. Thompson; Manuel A. Fernandes; Charles B. de Koning; Willem A. L. van Otterlo


Publisher
John Wiley and Sons
Year
2007
Tongue
English
Weight
223 KB
Volume
2007
Category
Article
ISSN
1434-193X

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✦ Synopsis


Abstract

The synthesis of 3‐methyl‐ and 3,4‐dimethyltetrahydroisoquinolines from aromatic aminoalkenes using intramolecular hydroamination reactions is described. This reaction was achieved by way of a reductive aminomercuration using mercuric acetate followed by sodium borohydride, or by using sub‐stoichiometric amounts of n‐butyllithium. (© Wiley‐VCH Verlag GmbH & Co. KGaA, 69451 Weinheim, Germany, 2007)