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Intracavity transient absorption effect on lasing of a dye-doped microspherical particle

✍ Scribed by Kenji Kamada; Keiji Sasaki; Hiroshi Masuhara


Publisher
Elsevier Science
Year
1994
Tongue
English
Weight
476 KB
Volume
229
Category
Article
ISSN
0009-2614

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✦ Synopsis


The effect of transient absorption on a lasing process occurring in a spherical particle was studied by use of a microspectroscopy system combined with a laser trapping technique. Stimulated emission of rhodamine B within a poly(methy1 methacrylate) latex particle was greatly attenuated by transient absorption of 9, lo-diphenylanthracene simultaneously doped in the particle. Compared with the absorption loss caused by a single path through the particle, the change in the lasing emission intensity was amplified by the optical resonance in a spherical microparticle by two orders of magnitude. The linearity of the emission intensity change with the intracavity transient absorption was also discussed. A new, sensitive method of transient absorption measurement based on the resonance effect is proposed for elucidating picosecond dynamics of a single microparticle.