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Interaction of remote functional groups (amide and amine) in steroidal compounds after electron ionization

✍ Scribed by Pierre Longevialle; Guy Bouchoux; Yannik Hoppilliard


Book ID
102965843
Publisher
John Wiley and Sons
Year
1990
Tongue
English
Weight
629 KB
Volume
25
Category
Article
ISSN
1076-5174

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✦ Synopsis


Electron impact ionization of steroidal compounds with two differently substituted functional groups (amide and amine) at remote positions leads to the interaction of these groups in ion-neutral complexes after the detachment of one of them. Two situations may be encountered, depending on which group is more easily detached from low-energy parent ions: (i) when the formation of the immonium ion is preferred, a very efficient proton transfer to the amide is observed leading to abundant [ Mimine]" and subsequent daughter ions; (ii) when the detachment of the amide is preferred, hydrogen exchanges occur with the amine group, and fragment ions may be observed resulting from the addition of both groups in a proton-bound structure.