Intensity and polarization of light emitted in slow ion-atom collisions
โ Scribed by Herbert F. M. Dacosta; David A. Micha; Keith Runge
- Publisher
- John Wiley and Sons
- Year
- 1996
- Tongue
- English
- Weight
- 531 KB
- Volume
- 60
- Category
- Article
- ISSN
- 0020-7608
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โฆ Synopsis
We study the intensity and polarization of light emitted during slow ion-atom collisions. We describe the nuclei as moving along classical trajectories while the electronic rearrangement is treated using time-dependent molecular orbitals. The intensity of emitted light is calculated from the diatomic time-dependent dipole. We evaluate the diatomic dipole matrix elements involving 1 s, 2 s, and 2 p traveling atomic orbitals suitable for time-dependent collision studies. We calculate the intensity and the polarization of light emitted in p + H(ls) collisions at kinetic energies from 10 to 1000 eV, for several impact parameters, changing over time. The emitted intensity goes through a maximum as the collision energy increases and lasts between 10 and 1 fs; the polarized light components parallel and perpendicular to the incoming beam direction show pronounced dependences on impact parameters and time.
๐ SIMILAR VOLUMES
Slow ionแatom collisions can be described within a first-principles molecular dynamics based on eikonal wave functions for the nuclei and the time-ลฝ . dependent HartreeแFock TDHF approximation for electrons that self-consistently couples the electronic and nuclear degrees of freedom. By expanding th
State-selective, non-dissociative electron capture processes by very slow nitrogen dications from atoms (He, Ne and Ar) and molecules (D2, N2 and O2) has been studied experimentally at impact energies of 28 eV by means of ion translational energy spectrometry and theoretically by means of ab initio