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Insights Into the Carbene-Initiated Aggregation of [Fe(cot)2]

✍ Scribed by Dr. Vincent Lavallo; Prof. Amer El-Batta; Prof. Guy Bertrand; Prof. Robert H. Grubbs

Book ID: 101571134
Publisher: John Wiley and Sons
Year: 2010
Tongue: English
Weight: 376 KB
Volume: 50
Category: Article
ISSN: 0044-8249
DOI: 10.1002/anie.201005212

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## Abstract Electrochemical investigations on a structural analogue of the [2Fe]~H~ subsite of [FeFe]H~2~ases, namely, [Fe~2~(CO)~6~{μ‐SCH~2~N(CH~2~CH~2~‐ OCH~3~)CH~2~S}] (1), were conducted in MeCN/NBu~4~PF~6~ in the presence of HBF~4~/Et~2~O or HOTs. Two different catalytic proton reduction proce