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Influence of Ionic and Polar Solutes upon ΔG≠ and ΔV≠ of the Amide Rotation in Aqueous Solutions of Dimethylacetamide

✍ Scribed by Dr. Gerhard Völkel; Dipl.-Phys. Johann Hauer; Prof. Dr. Hans-Dietrich Lüdemann


Publisher
John Wiley and Sons
Year
1980
Tongue
English
Weight
240 KB
Volume
19
Category
Article
ISSN
0044-8249

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✦ Synopsis


As a probe for changes in hydrate structure one can use the pressure‐dependence of the activation volume Δ__V__^≠^ for rotation of the Me~2~N group in dimethyl acetamide (DMA). In dilute solutions Δ__V__^≠^ for DMA is practically pressure‐independent, but is increased by ionic solutes. This could indicate an open hydrate sheath in which the rotation can take place without the water molecules in the surroundings being re‐ordered.