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“Increased-valence” bonding units: 6-electron 5-centre bonding for S4N4, pyrrole and Xe2F3+ and the π-bonding for S4N3+, S2N2 and (SN)x

✍ Scribed by R.D Harcourt

Book ID
115974517
Publisher
Elsevier Science
Year
1977
Weight
482 KB
Volume
39
Category
Article
ISSN
0022-1902

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A study of the electronic structures of
A study of the electronic structures of SN, S2N2, S4N4, NO, and N2O2 and their implications for (SN)x
✍ Salahub, D. R. 📂 Article 📅 1976 🏛 American Institute of Physics 🌐 English ⚖ 796 KB

SCF–Xα–SW calculations have been carried out for SN, S2N2, and S4N4 as well as the analogous oxides NO and N2O2. The electronic charge distribution of the sulfides is remarkably uniform leading to highly polar SN bonds (∼S+1/2N−1/2) in contrast to the oxides where the NO bonds involve less charge tr