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In situ Raman spectra of the discharge products of calcium and lithium-anoded thionyl chloride cells — sulphur dioxide generation in oxyhalide systems

✍ Scribed by W.P. Hagan; D.G. Sargeant


Publisher
Elsevier Science
Year
1991
Tongue
English
Weight
640 KB
Volume
34
Category
Article
ISSN
0378-7753

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✦ Synopsis


A cell has been constructed that allows a caknun or hthmm-anoded oxyhahde cell of conventional composition to be analysed for catholyte-soluble &charge products usmg laser Raman spectroscopy Both cells showed the presence of sulphur dloxlde solvated by tluonyl chlonde Speaes of the type M(SOCl,)(SOJ'+(AlCl,),-could only be detected III cells havmg calcmm or l~thnun anodes w&h LuIlCI, as the supportmg electrolyte m 0uonyl chlonde Vapour pressure measurements of dwchargmg cells co-ed that Ca(AlCl& was less hkely to form a complex with sulphur &oxlde than the analogous hthnun salt