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Improving GC-MS screening analysis by functional-group-related silica gel fractionation of industrial wastewater extracts

✍ Scribed by Reemtsma, Thorsten ;Jekel, Martin


Publisher
John Wiley and Sons
Year
1994
Tongue
English
Weight
504 KB
Volume
17
Category
Article
ISSN
0935-6304

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✦ Synopsis


Abstract

The separation of the components of complex industrial waste water extracts according to their functional groups has been accomplished by use of small silica gel columns eluted with a hexane – dichloromethane – methanol gradient. The six fractions obtained covered a polarity range from aliphatic fatty acids to (aromatic) polyhydroxy and polyether compounds. Recovery of model compounds was between 75 and 105%.

Used prior to GC‐MS analysis this fractionation substantially enhances chromatographic resolution and facilitates peak identification. The procedure was exemplarily applied to an extract of anaerobically treated tannery waste water. Phenols, aromatic acids, and aromatic and aliphatic (poly)hydroxy acids, in the low ppm range, were determined as main constituents. Since fractionation extends the range of detection, trace substances such as chlorocresol, dichlorobenzoic acid, mercaptobenzothiazole, and mercaptoacetic acid were also detectable at the ppb level.