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Identity of 3,4-dimethylenethiophene reactive intermediates from diazene and bis-allene precursors. Correlation of singlet biradical reactivity in the tetramethyleneethane and trimethylenemethane series.

✍ Scribed by Marc M. Greenberg; Silas C. Blackstock; Jerome A. Berson


Publisher
Elsevier Science
Year
1987
Tongue
French
Weight
253 KB
Volume
28
Category
Article
ISSN
0040-4039

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✦ Synopsis


The relative reactivities of the 3,4_dimethylenethiophene intermediates 1 from the deazetation of the diazene 5 and from the intramolecular cyclization of bisallenyl sulfide 3, determined by competition experiments, serve as a "fingerprint" to show that the same reactive transient is generated from both precursors.