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Hydrogen Dissociation and Spillover on Individual Isolated Palladium Atoms

✍ Scribed by Tierney, Heather L.; Baber, Ashleigh E.; Kitchin, John R.; Sykes, E. Charles H.

Book ID
121662797
Publisher
The American Physical Society
Year
2009
Tongue
English
Weight
795 KB
Volume
103
Category
Article
ISSN
0031-9007

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A portion of the hydrogen of a high-surface-area silica was exchanged with deuterium gas in a pulse flow microreactor. The exchange reaction was rapid at 190 β€’ C when the silica was physically mixed with a Pd on carbon catalyst. The amount of readily exchangeable hydrogen was determined using a titr