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Homogeneous catalysis. Use of the [TiCp2(CF3SO3)2] catalyst for the sakurai reaction of allylic silanes with orthoesters, acetals, ketals and carbonyl compounds.

✍ Scribed by T.Keith Hollis; N.P. Robinson; John Whelan; B. Bosnich


Publisher
Elsevier Science
Year
1993
Tongue
French
Weight
297 KB
Volume
34
Category
Article
ISSN
0040-4039

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✦ Synopsis


The effectiveness of the [TiCp2(CF$O3)2] catalyst for the Sakurai reaction has been exploredfor a variety of allylic silanes reacting with orthoesters, ace&, ketals, aldehydes and ketones.

The Sakurai reaction (eqs 1.2) is promoted by a variety of Lewis acid@ including TiQ, Alc13, BF3, MesSi R' IF0 + "esiMe3 __) Rh-(l)