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Hole-burning spectra of the isomeric forms of jet-cooled anthracene complexes with aniline derivatives

✍ Scribed by F. Piuzzi


Publisher
Elsevier Science
Year
1993
Tongue
English
Weight
739 KB
Volume
209
Category
Article
ISSN
0009-2614

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✦ Synopsis


Fluorescence-excitation spectra and hole-burning spectra are recorded for jet-cooled complexes of anthracene with dimethylaniline (DMA) and dimethyl-ptoluidine (DMPT). The existence of isomeric forms (two in the first and three in the latter case) is evidenced. One of these forms (E form) showing broad-band absorption and exciplex-like emission spectra probably corresponds to a stacked configuration of donor and acceptor molecules. The T-shaped and stacked/displaced configurations are proposed for the forms R characterized by narrow-band absorption and resonant fluorescence. The relation between the excited-state isomerization threshold and the IVR onset is discussed.