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High-throughput screening of optimal solution conditions for structural biological studies by fluorescence correlation spectroscopy

✍ Scribed by Toshihiko Sugiki; Chie Yoshiura; Yutaka Kofuku; Takumi Ueda; Ichio Shimada; Hideo Takahashi


Book ID
105356783
Publisher
Cold Spring Harbor Laboratory Press
Year
2009
Tongue
English
Weight
280 KB
Volume
18
Category
Article
ISSN
0961-8368

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✦ Synopsis


Abstract

Protein aggregation is an essential molecular event in a wide variety of biological situations, and is a causal factor in several degenerative diseases. The aggregation of proteins also frequently hampers structural biological analyses, such as solution NMR studies. Therefore, precise detection and characterization of protein aggregation are of crucial importance for various research fields. In this study, we demonstrate that fluorescence correlation spectroscopy (FCS) using a single‐molecule fluorescence detection system enables the detection of otherwise invisible aggregation of proteins at higher protein concentrations, which are suitable for structural biological experiments, and consumes relatively small amounts of protein over a short measurement time. Furthermore, utilizing FCS, we established a method for high‐throughput screening of protein aggregation and optimal solution conditions for structural biological experiments.