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Generalised relations for the thermal diffusion factor of inert gas mixtures with one invariable constituent

✍ Scribed by B.N. Srivastava; S.C. Saxena


Publisher
Elsevier Science
Year
1956
Weight
481 KB
Volume
22
Category
Article
ISSN
0031-8914

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✦ Synopsis


The variation of the thermal diffusion factor c~ for binary mixtures of inert gases, when one constituent is kept fixed and the other varied, has been investigated and semi-empirical formulae have been derived for the variation of c¢ with the proportionate mass difference of the molecules. These results have been explained in terms of the Chapman-Enskog formula for the case of Lennard-Jones 12 : 6 model by utilising the experimentally obtained unique dependence of the force constants Ei~. and r;j on the molecular mass of the variable constituent for a given series of mixtures. The same considerations have been applied to isotopes of monatomic molecules and suitable formulae have been deduced for c~, en and r n. The formulae have been tested by calculating the force constants of radon.