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Gaussian basis sets for use in correlated molecular calculations. VIII. Standard and augmented sextuple zeta correlation consistent basis sets for aluminum through argon

✍ Scribed by Tanja Van Mourik; Thom H. Dunning Jr.


Publisher
John Wiley and Sons
Year
2000
Tongue
English
Weight
399 KB
Volume
76
Category
Article
ISSN
0020-7608

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✦ Synopsis


Standard and augmented correlation consistent sextuple zeta cc-pV6Z

. and aug-cc-pV6Z basis sets have been determined for the second-row atoms aluminum through argon. Using these sets, dissociation energies and spectroscopic constants for the ground states of HCl, PN, and P have been calculated using several theoretical methods, 2 including Møller᎐Plesset perturbation theory, coupled cluster theory, and multireference Ž . configuration interaction theory MRCI . The aug-cc-pV6Z and cc-pV6Z sets yield dissociation energies that are estimated to be within 0.1᎐0.2 kcalrmol of the complete Ž . basis set limit for HCl and within 1᎐1.5 kcalrmol for PN and P . The MRCI and CCSD T 2 methods are found to give the most consistently reliable results for the spectroscopic