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Functionalization of PAMAM dendrimers with nitronyl nitroxide radicals as models for the outer-sphere relaxation in dentritic potential MRI contrast agents

✍ Scribed by Giancarlo Francese; Frank A. Dunand; Claudia Loosli; André E. Merbach; Silvio Decurtins


Publisher
John Wiley and Sons
Year
2003
Tongue
English
Weight
164 KB
Volume
41
Category
Article
ISSN
0749-1581

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✦ Synopsis


Abstract

PAMAM dendrimers functionalized with nitronyl nitroxide radicals were characterized. Quantitative determination of substitution with radicals was performed using EPR and electrochemical methods. The study of the ^1^H NMR relaxation of the surrounding water showed how the outer‐sphere contribution to the relaxivity may be limited by the presence of the dendrimer core. Copyright © 2003 John Wiley & Sons, Ltd.