The present work demonstrates that the number of scattering problems which can be handled accurately by the semiclassical (thawed) Gaussian method can be increased substantially if the calculations are done within the framework of the interaction picture. Examples for photodissociation of three atom
Fragments in Gaussian wave-packet dynamics with and without correlations
✍ Scribed by Dieter Kiderlen; Paweł Danielewicz
- Publisher
- Elsevier Science
- Year
- 1997
- Tongue
- English
- Weight
- 951 KB
- Volume
- 620
- Category
- Article
- ISSN
- 0375-9474
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✦ Synopsis
Generalization of Gaussian trial wave functions in quantum molecular dynamics models is introduced, which allows for long-range correlations characteristic for composite nuclear fragments. We demonstrate a significant improvement in the description of light fragments with correlations. Utilizing either type of Gaussian wave functions, with or without correlations, however, we find that we cannot describe fragment formation in a dynamic situation. Composite fragments are only produced in simulations if they are present as clusters in the substructure of original nuclei. The difficulty is traced to the delocalization of wave functions during emission. Composite fragments are produced abundantly in the Gaussian molecular dynamics in the limit h ~ 0.
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