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Fractal to classical crossover of chemical reactions

✍ Scribed by J.S. Newhouse; P. Argyrakis; R. Kopelman

Publisher
Elsevier Science
Year
1984
Tongue
English
Weight
347 KB
Volume
107
Category
Article
ISSN
0009-2614

No coin nor oath required. For personal study only.

✦ Synopsis

Computer simulations on binary reactions of random walkers (A + A -A) on two-and three-dimensional percohtion clusters bear out the recent superuniversality conjecture (integrated reaction rate 0~ f 2f3). nitmover. the fr~ct&to+uclide3n crossover (r2'3 to t dependence) pantfels that of the single watker.

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The Bessel uniform approximation developed by Stine and Marcus is applied to the collinear H f Hz reaction on Diestler's potential energy surface no. 3 to which we have' previously applied other orders of approximation of classicai S matrix theory. It appears that an accurate treatment of this syste