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Fourier transform millimeter-wave spectroscopy of CS(X1Σ+) and SO(b1Σ+) in highly excited vibrational states

✍ Scribed by Eunsook Kim; Satoshi Yamamoto

Publisher: Elsevier Science
Year: 2003
Tongue: English
Weight: 170 KB
Volume: 219
Category: Article
ISSN: 0022-2852
DOI: 10.1016/s0022-2852(03)00027-4

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✦ Synopsis

The rotational spectral lines of CS(X 1 R þ ) and SO(b 1 R þ ) in the highly excited vibrational states have been observed with the Fourier transform millimeter-wave spectrometer in combination with a pulsed discharge nozzle. The

are detected for several vibrational states. These measurements lead to a precise determination of the Dunham coefficients. In addition to the normal species, the spectral lines of their isotopomers have also been observed. The hyperfine interaction constants of 13 CS and C 33 S are determined in each excited vibrational state. The present measurements indicate that the pulsed discharge nozzle system can produce a molecule in highly excited vibrational states as well as in the metastable electronic states.

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