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Formation of six carbon-carbon bonds in a one pot process. Generation of the dicyclopenta[a,e]pentalene ring system via the tandem Pauson-Khand reaction

โœ Scribed by Scott G. Van Ornum; James M. Cook

Publisher
Elsevier Science
Year
1997
Tongue
French
Weight
108 KB
Volume
38
Category
Article
ISSN
0040-4039

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โœฆ Synopsis

The regiospecific synthesis of the four five-membered rings of a suitably functionalized parent system 11 of dicyclopenta[a,e]pentalene 2 has been accomplished via a tandem Pauson-Khand reaction in a one pot process.

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The livinghouse catalytic approach to the tandem Pauson-Khand reaction. Entry into the parent ring systems of dicyclopenta[a,f]pentalene and dicyclopenta[a,e]pentalene
โœ Scott G. Van Ornum; Michelle M. Bruendl; James M. Cook ๐Ÿ“‚ Article ๐Ÿ“… 1998 ๐Ÿ› Elsevier Science ๐ŸŒ French โš– 111 KB

The first photochemically-mediated catalytic tandem Pauson-Khand reaction has permitted the preparative scale synthesis of the parent ring systems 4 and 6 of dicyclopenta[a,f]pentalene 1 and dicyclopenta[a,e]pentalene 2, respectively.