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Formation of epitaxial β-SiC layers by fullerene-carbonization of silicon(001): a comparison between the use of C60 and C70 molecules

✍ Scribed by S. Henke; M. Philipp; B. Rauschenbach; B. Stritzker


Publisher
Elsevier Science
Year
1996
Tongue
English
Weight
301 KB
Volume
36
Category
Article
ISSN
0921-5107

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✦ Synopsis


By condensation of C6o and C7o fullerenes the formation of continuous, thick epitaxial t-SiC films on Si(001) and Si(lll) surfaces is possible, even at moderate temperatures (700 °C-1000 °C). The dependence of structure, topography, and composition of the epitaxial silicon carbide layers formed by C6o or C70 carbonization of silicon on the substrate temperature was studied by X-ray diffraction, atomic force microscopy, and Rutherford-backscattering analysis. It could be shown that the quality of the formed epitaxial t-SiC layers is extremely sensitive to the substrate temperature. In the case of C60 and a substrate temperature of 850 °C the growth of epitaxial t-SiC layers with only a small number of defects was observed. Lowering the substrate temperature to 775 °C resulted in t-SiC layers with a strong texture. Using C70 molecules the process temperature can be lowered further by 75 °C. High quality t-SiC layers with a low number of defects can be grown at a substrate temperature of as low as 775 °C.