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Fluorescent PET (photoinduced electron transfer) indicators for solvent polarity with quasi-step functional response

✍ Scribed by Richard A. Bissell; A.Prasanna de Silva; W. Thilak; M.L. Fernando; Suram T. Patuwathavithana; T.K. Shantha; D. Samarasinghe


Book ID
104225419
Publisher
Elsevier Science
Year
1991
Tongue
French
Weight
304 KB
Volume
32
Category
Article
ISSN
0040-4039

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✦ Synopsis


The family of alkylaminomethylanthracenes

(1) display solvent independent electronic spectral parameters except for the fluorescence quantum yield which gives a sharp sigmoidal response to solvent polarity.The latter can he analyzed according to a linear free energy relationship. Photophysical studies of aromatic hydrocarbon-amine systems have demonstrated solvent polarii,y dependent photoinduced electron transfer (PET) and exciplex emission. 1 Exciplex emission is largely suppresF(:d by a) the presence of two aliphatic amine units2, b) the restricted geometric relationship of hydrocarbon and amine in intramolecular situations caused by a single methylene spacer3, and (c) the presence of N-H bonds.4 We now