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Flexibility of a labeled polymer chain: Time-resolved fluorescence depolarization measurements and their interpretation by a Hinged-Dumbbell model

✍ Scribed by J. Ricka; K. Amsler; Th. Binkert


Publisher
Wiley (John Wiley & Sons)
Year
1983
Tongue
English
Weight
993 KB
Volume
22
Category
Article
ISSN
0006-3525

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✦ Synopsis


Time-resolved fluorescence depolarization was applied to investigate the dynamics of low-molecular-weight polyethylene glycols ( M W 150, 400, 1000, 4000) labeled by fluorescein-isothiocyanate. The analysis of measurements revealed considerable flexibility of the polymer chain. To interpret the observed dependence of the relaxation time of polarization anisotropy on the molecular weight of the polymer, a simple freely-hinged dumbbell model was developed. The properties of the model were investigated by computer experiments.