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Fe[5NO2-sal-N(1,4,7,10)]: a new iron(II) complex exhibiting an unusual two-step spin conversion afforded by a hexadentate ligand with a N4O2, donor set

✍ Scribed by V. Petrouleas; J.-P. Tuchagues


Publisher
Elsevier Science
Year
1987
Tongue
English
Weight
384 KB
Volume
137
Category
Article
ISSN
0009-2614

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✦ Synopsis


The new Fe[ SNO,-sal-N( 1,4,7, IO)] spin-crossover complex'has been investigated by Miissbauer spectroscopy, magnetic susceptibility measurements, and X-ray diffraction powder studies as a function of temperature. The spin conversion occurs in two steps separated by a 30" broad spin equilibrium domain involving 50% of HS and LS complex molecules. A single structural phase characterizes this complex from 300 to 90 K. This is the first iron( II) spin-crossover complex including a N,O, donor set.