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Fast Deswelling Kinetics of Nanostructured Poly(N-Isopropylacrylamide) Photopolymerized in a Lyotropic Liquid Crystal Template

✍ Scribed by Bradley S. Forney; C. Allan Guymon


Book ID
102497603
Publisher
John Wiley and Sons
Year
2011
Tongue
English
Weight
274 KB
Volume
32
Category
Article
ISSN
1022-1336

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✦ Synopsis


Abstract

The thermal‐response and mechanical properties of poly(N‐isopropylacrylamide) (PNIPAm) are improved by controlling the polymer nanostructure through photopolymerization in a bicontinuous cubic lyotropic liquid crystal (LLC) template. The bicontinuous cubic nanostructure increases the rate and amount of water expelled from PNIPAm for heating above the lower critical solution temperature (LCST) relative to an isotropic PNIPAm hydrogel while maintaining the mechanical integrity of the polymer. These results could allow development of PNIPAm hydrogels with proper water uptake, deswelling kinetics, volume transition, and mechanical properties required for successful performance in a growing number of advanced biological and industrial applications. magnified image