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Facile Access to an Efficient Solid-Supported Click Catalyst System Based on Poly(ethyleneimine)

✍ Scribed by Lies Bonami; Wim Van Camp; Dieter Van Rijckegem; Filip E. Du Prez


Publisher
John Wiley and Sons
Year
2009
Tongue
English
Weight
227 KB
Volume
30
Category
Article
ISSN
1022-1336

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✦ Synopsis


Abstract

A novel heterogeneous copper(I) catalyst system, which is based on readily available poly(ethyleneimine), has been used as a recyclable catalyst for Cu(I) catalyzed “click” 1,3 dipolar cycloaddition reactions of azides and alkynes in organic media. Branched poly(ethyleneimine) was first methylated and then cross‐linked with 1,9‐dibromononane. Subsequently, after the immobilization of Cu(I)Br, this system was applied for heterogeneous copper catalyzed click chemistry of a few model reagents and polymeric compounds.

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