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Experimentally-validated micromixing-based CFD model for fed-batch stirred-tank reactors

✍ Scribed by Otute Akiti; Piero M. Armenante


Publisher
American Institute of Chemical Engineers
Year
2004
Tongue
English
Weight
246 KB
Volume
50
Category
Article
ISSN
0001-1541

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✦ Synopsis


Abstract

A model was developed to predict the final product distribution in fed‐batch, stirred‐tank reactors carrying out fast, parallel, chemical reactions, and the predictions were compared with experimental data. The following reaction system was chosen:

equation image

Comparison between the experimentally determined flow field inside the reactor, obtained with a laser‐doppler velocimeter (LDV), and the predictions from computational fluid dynamics (CFD) simulations was favorable. A model was developed to predict the yield, X~S~, of forming S from A, using CFD to describe the velocity distribution inside the reactor, two micromixing models to represent the interaction between turbulence effects and chemical reactions, and a multiphase model (Volume of Fluid (VOF) model) to track the reacting zone in a Lagrangian fashion. Model predictions for X~S~ were compared with experimental data. The agreement between the experiments and the results of the simulations was good. © 2004 American Institute of Chemical Engineers AIChE J, 50:566–577, 2004