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Examination of an “improved” cell theory

✍ Scribed by D.J. Adams; A.J. Matheson

Publisher
Elsevier Science
Year
1973
Tongue
English
Weight
349 KB
Volume
22
Category
Article
ISSN
0009-2614

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✦ Synopsis

The simpk ~~11 theory of dense simple liquids, based on irregularly arranged cells, is exrended by allowing the atoms in a11 the cells to bchavc in the same fashion as the "reference" atom. It is shown that such a modification leads to two widely different sets ot rherrnodynamic predictions, one of which is a modest improvement over the results of the original theory. The thermodynamic inconsistency is a result of the cell field potential being a function of temperature. A necessary cc?dition which any cell theory of this general type must obey in order to have thermodynamic consistency is given.

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