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Evidence from Circular Dichroism and from Melting Behavior for Helix-Inducing Complexation of a Designed β3-Pentadecapeptide with DNA Duplexes. Preliminary Communication

✍ Scribed by Thierry Kimmerlin; Kenji Namoto; Dieter Seebach


Publisher
John Wiley and Sons
Year
2003
Tongue
German
Weight
152 KB
Volume
86
Category
Article
ISSN
0018-019X

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✦ Synopsis


Abstract

Inspired by naturally occurring DNA‐binding proteins and their artificial α‐peptidic mimics reported to date, a research project was initiated aiming at creating a new class of β‐peptides capable of binding to and ultimately regulating the functions of DNA. As an initial foray, a β^3^‐pentadecapeptide 1, which bears H‐bonding Asn side chains and positively charged Lys side chains, was designed and synthesized on the solid support. DNA‐Complexation studies by means of circular dichroism and DNA‐melting‐temperature measurements revealed the first preliminary indications that support the existence of ordered interactions between β‐peptides and DNA.