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Enhanced resolution in the 1H NMR spectra of zeolite H-ZSM-5 by heteronuclear dipolar-dephasing spin-echo MAS

✍ Scribed by Dieter Freude


Publisher
Elsevier Science
Year
1995
Tongue
English
Weight
513 KB
Volume
235
Category
Article
ISSN
0009-2614

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✦ Synopsis


Dipolar-dephasing with high power 2~M irradiation yields 1H MAS NMR echo spectra of 'aluminium-unconnected' hydroxyl groups in dehydrated zeolites. The aluminium-connected SiOHAI and AIOH hydroxyls can be observed as the difference spectra. The technique increases the number of OH lines in the 1H NMR spectra of dehydrated zeolite H-ZSM-5. Two kinds of Brcnsted sites can be distinguished and interpreted in terms of their mobility in the vicinity of framework aluminium atoms.