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Energy-Transfer Modeling for the Rational Design of Multiporphyrin Light-Harvesting Arrays

โœ Scribed by Van Patten, P. Gregory; Shreve, Andrew P.; Lindsey, Jonathan S.; Donohoe, Robert J.

Book ID
121354725
Publisher
American Chemical Society
Year
1998
Tongue
English
Weight
157 KB
Volume
102
Category
Article
ISSN
0022-3654

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ฯ€-Electronic conjugation is not necessary to facilitate long-range energy migration and transfer: A rapid (k =1.04ร—10 s ) and efficient (ฮฆ =71โ€‰%) energy transfer from the 28 photoexcited zinc porphyrin units to the focal free-base porphyrin unit occurs in a large, star-shaped dendritic multiporphyri