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Enantioselective Synthesis of Oasomycin A, Part I: Synthesis of the C1–C12 and C13–C28 Subunits

✍ Scribed by David A. Evans; Pavel Nagorny; Kenneth J. McRae; Dominic J. Reynolds; Louis-Sebastian Sonntag; Filisaty Vounatsos; Risheng Xu

Publisher: John Wiley and Sons
Year: 2007
Tongue: English
Weight: 240 KB
Volume: 119
Category: Article
ISSN: 0044-8249
DOI: 10.1002/ange.200603653

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Scheme 1. Retrosynthetic analysis of oasomycin A. Bn = benzyl.

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The first members of the pectenotoxin family of marine natural products were isolated off the northeastern coast of Japan in 1985. Subsequently, ten members of this group have been identified. The structural diversity within the pectenotoxins stems from variations in the oxidation state at C43, as