Emission in CS2 vapor stimulated by a counterintuitive sequence of pulses
β Scribed by V. Khidekel; B. Fain; H.T. Liou; S.H. Lin
- Publisher
- Elsevier Science
- Year
- 1995
- Tongue
- English
- Weight
- 431 KB
- Volume
- 234
- Category
- Article
- ISSN
- 0009-2614
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β¦ Synopsis
Measurement of the stimulated emission from a cell containing CS2 molecules irradiated by two laser pulses is discussed. Both an approximate adiabatic solution and an exact numerical solution have been used to explain the results. It has been proved that, to obtain maximal signal, the pulses must come to the cell in a counterintuitive order, that is, the stimulating pulse arrives prior to the pump pulse. The connection with the phenomenon of efficient population transfer has been pointed out.
π SIMILAR VOLUMES
The relaxation of single vibrational levels of CS2 (R 3B2) has been studied by the stimulated emission pumping technique for the first time. The relaxation rate of the 0,6,0 and 0,8,0 levels is found to be 0.89x lOa s-r TOK-' and 1.2x 10' s-r Tow' respectively. These values are about an order of mag
The (Z]"ll,+x 'z transition of Cs2 is observed in a very cold pulsed molecular beam using the resonanceenhanced twophoton ionization method. The term values ofthe substates of (2)'l&state are determined tobe T,= 14121.OkO. 1,14013.2 f 0.1, 13912.9+0. I, and 13909.4f 0.1 cm-' for the 2, l,, O,+, and