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Electron transfer photochemistry of bridged allylcyclopropane systems: novel substitution products via deprotonation

✍ Scribed by Dahui Zhou; Jolene Chou; Heinz D. Roth


Publisher
John Wiley and Sons
Year
1999
Tongue
English
Weight
107 KB
Volume
12
Category
Article
ISSN
0894-3230

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✦ Synopsis


The electron transfer photochemistry of three rigid, bridged allylcyclopropane systems, 3-carene (1), tricyclo[4.3.1.0 1,6 ]dec-3-ene (2) and tricyclo[4.4.1.0 1,6 ]undeca-3,8-diene (3), is shown to take an unprecedented course: the major products are novel 'substitution' products, in which a hydrogen at an allylic carbon (C 2 ) of the substrate has been replaced by the p-cyanophenyl group.