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Electron Transfer Mechanism in Helical Peptides

✍ Scribed by Mandal, Himadri Shekhar; Kraatz, Heinz-Bernhard

Book ID
120243040
Publisher
American Chemical Society
Year
2012
Tongue
English
Weight
893 KB
Volume
3
Category
Article
ISSN
1948-7185

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## Abstract Helical peptides of 8mer, 16mer, and 24mer carrying a disulfide group at the __N__‐terminal and a ferrocene moiety at the __C__‐terminal were synthesized, and they were self‐assembled on gold by a sulfur–gold linkage. Infrared reflection–absorption spectroscopy and ellipsometry confirme

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The ␣-helical structure of donor-acceptor-substituted peptides 1 and 2 was established by circular dichroism and NMR spectroscopy. The photoproduction of a spatially separated radical ion pair was detected by transient absorption spectroscopy. The expected influence of the electric field along the h