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Electric field effects on zero-kinetic-energy photoelectron spectra: An explanation of observed trends

✍ Scribed by F. Merkt; H.H. Fielding; T.P. Softley


Publisher
Elsevier Science
Year
1993
Tongue
English
Weight
725 KB
Volume
202
Category
Article
ISSN
0009-2614

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✦ Synopsis


An explanation is offered for the propensity for large negative changes of rotational angular momentum in ZEIG photoelectron spectra, which is increasingly observed as the rotational constant of the photoion decreases; Stark mixing becomes progressively more important, facilitating multistep rotational autoionization processes. The Inglis-Teller limit serves as a useful benchmark for assessing the importance of electric field effects. A discussion is presented of the relative importance of I mixing and Jmixing.