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Efficient control of electron localization by subcycle waveform synthesis

✍ Scribed by Lan, Pengfei; Takahashi, Eiji J.; Midorikawa, Katsumi

Book ID: 115311542
Publisher: The American Physical Society
Year: 2012
Tongue: English
Weight: 920 KB
Volume: 86
Category: Article
ISSN: 1050-2947
DOI: 10.1103/physreva.86.013418

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## Abstract (±)‐Modhephene (**6**) has been synthesized from the easily available trimethylpentalenone **1** in 6 steps in 26% overall yield __(Scheme 2)__. The remarkably smooth 1,4‐addition/enolate trapping **1** → **2** and subsequent selenoxide elimination after oxidation furnished the key inte